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Regular Paper

Manufacturing Process Optimization of Oxide-Based Multilayer Ceramic Batteries Using Multilayer Ceramic Processing Technologies
Won-Su Lee, Jong Kyu Lee, Jung Rag Yoon
J Electr Electron Mater 2026;39(5):519-531.
Published online September 1, 2026
DOI: https://doi.org/10.4313/JEEM.2026.39.5.9
Multilayer ceramic batteries (MLCBs) have attracted increasing attention as compact all-solid-state energy-storage devices that can be manufactured using multilayer ceramic processing technologies. In this study, an MLCC-compatible fabrication process for oxide-based MLCBs was developed using Li₁₊ₓAlₓTi₂₋ₓ(PO₄)₃ (LATP) solid electrolytes, Li₃V₂(PO₄)₃ (LVP) cathodes, and Cu current collectors. Commercial LATP powders were evaluated in terms of particle-size distribution, phase purity, thermal stability, and ionic conductivity. The selected LATP powder was subsequently employed for tape-cast green-sheet fabrication, and the effects of polyvinyl butyral (PVB) binder content on slurry rheology and sheet microstructure were investigated. An optimized binder composition containing 11 wt% PVB (BM-2/BH-3 = 3:7) provided improved processability and microstructural uniformity. Drying conditions during sequential electrode printing were also optimized to suppress sheet warpage and improve multilayer registration. Thermogravimetric and differential thermal analyses (TG–DTA) were used to establish an optimized two-step debinding and co-firing process under a controlled reducing atmosphere. The resulting multilayer structures exhibited uniform densification without significant blistering, delamination, or interfacial defects. Charge–discharge measurements confirmed that electrochemical functionality was retained after the complete manufacturing process, yielding a discharge capacity of approximately 2.5–2.7 μAh.
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The Analysis on the Effect of Improving Aspect Ratio and Electrode Spacing of the Crystalline Silicon Solar Cell
Min Young Kim, Ju Eok Park, Hae Sung Cho, Dae Sung Kim, Seong Kyun Byeon, Dong Gun Lim
J Korean Inst Electr Electron Mater Eng 2014;27(4):209-216.   Published online April 1, 2014
DOI: https://doi.org/10.4313/JKEM.2014.27.4.209
The screen printed technique is one of the electrode forming technologies for crystalline silicon solar cell. It has the advantage that can raise the production efficiency due to simple process. The electrode technology is the core process because the electrode feature is given a substantial factor (for solar cell efficiency). In this paper, we tried to change conditions such as squeegee angle 55∼75°, snap off 0.5∼1.75mm, printing pressure 0.6∼0.3 MPa and 1.6∼2.0 mm finger spacing. As a result, the screen printing process showed an improved performance with an increased height higher finger height. Optimization of fabrication process has achieved 17.48% efficiency at screen mesh of 1.6 mm finger spacing.
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Energy Materials : Co-firing Optimization of Crystalline Silicon Solar Cell Using Rapid Thermal Process
Byoung Jin Oh, In Hwan Yeo, Dong Gun Lim
J Korean Inst Electr Electron Mater Eng 2012;25(3):236-240.   Published online March 1, 2012
DOI: https://doi.org/10.4313/JKEM.2012.25.3.236
Limiting thermal exposure time using rapid thermal processing(RTP) has emerged as promising simplified process for manufacturing of solar cell in a continuous way. This paper reports the simplification of co-firing using RTP. Actual temperature profile for co-firing after screen printing is a key issue for high-quality metal-semiconductor contact. The plateau time during the firing process were varied at 450℃ for 10~16 sec. Glass frit in Ag paste etch anti-reflection layer with plateau time. Glass frit in Ag paste is important for the Ag/Si contact formation and performances of crystalline Si solar cell. We achieved 17.14% efficiency with optimum conditions.
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